Office 365 - Outlook 2016 (How To) Clean Up Contact Groups
Outlook 2016 is the recommended client for cleaning up contact groups.
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With Outlook 2016 open, select People on the Navigation bar.
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In the My Contacts drop down menu on the left side of the screen, select the group from which you want to delete.
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The contacts will display in a list in the next pane.
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Deleting:
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Single Contact: Select a contact, press Delete on keyboard.
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Multiple Contacts, Non-contiguous: Select a contact, press and hold CTRL key while selecting additional contact(s), press Delete on keyboard.
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Multiple Contacts, Contiguous: Select a contact, Shift key while selecting last contiguous contact, press Delete on keyboard.